Researchers at the Technion – Israel Institute of Technology have developed a coherent and controllable spin-optical laser based on a single atomic layer. This discovery is enabled by coherent spin-dependent inter­actions between a single atomic layer and a laterally confined photonic spin lattice, the latter of which supports high-Q spin-valley states through the photonic Rashba-type spin splitting of a bound state in the continuum. The achievement paves the way to study coherent spin-dependent phenomena in both classical and quantum regimes, opening new horizons in fundamental research and opto­electronic devices exploiting both electron and photon spins.

The study was conducted in the research group of Erez Hasman, head of the Atomic-Scale Photonics Laboratory, in colla­boration with Elad Koren, head of the Laboratory for Nanoscale Electronic Materials and Devices in the Department of Materials Science and Engineering, and Ariel Ismach at Tel Aviv University. The two groups at the Technion are in association with the Helen Diller Quantum Center and Russell Berrie Nano­technology Institute (RBNI). Kexiu Rong conducted and led the research. According to Rong, “Spin-optical light sources combine photonic modes and electronic transitions and therefore provide a way to study the exchange of spin information between electrons and photons and to develop advanced opto­electronic devices.”

To construct these sources, a prerequisite is to lift the spin degeneracy between the two opposite spin states either in their photonic or electronic parts. This is usually accomplished by applying magnetic fields under a Faraday or Zeeman effect, although these approaches generally require strong magnetic fields and cannot produce miniaturized sources. Another promising way takes advantage of artificial magnetic fields for photonic spin-split states in momentum space, underpinned by a geometric phase mechanism. Unfor­tunately, previous observations of spin-split states have relied heavily on propagation modes with low quality factors, which impose undesired limitations on spatial and temporal coherence of the sources. This approach is also hindered by the spin-controllable properties of a bulk laser gain material being unavailable or nontrivial to access for active control of the sources, especially in the absence of magnetic fields at room tempera­ture.

To achieve high-Q spin-split states, the researchers constructed photonic spin lattices with different symmetry properties, which comprise an inversion-asymmetry core and inversion-symmetry cladding integrated with a WS₂ monolayer to create laterally confined spin-valley states. The essential inversion-asymmetry lattice the researchers use has two important properties. A controllable spin-dependent reciprocal lattice vector due to space-variant geometric phases from its constituting inhomo­geneous-anisotropic nanoholes. This vector splits a spin-degenerate band into two spin-polarized branches in momentum space, being referred to as the photonic Rashba effect. And a pair of high-Q symmetry-enabled (quasi-) bound states in the continuum, that is, ±K (corners of the Brillouin zone) photonic spin-valley states, at the band edges of the spin-split branches. Moreover, the two states form a coherent super­position state with equal amplitudes.

Koren noted that, “We used a WS₂ monolayer as the gain material because this direct-bandgap transition metal dichal­cogenide possesses unique valley pseudospins, which have been widely investigated as an alternative information carrier in valleytronics. Specifically, their ±K' valley excitons – radiated as in-plane spin-polarized dipole emitters – can be selectively excited by spin-polarized light according to a valley-contrasted selection rule, thus enabling active control of spin-optical light sources without magnetic fields.”

In the monolayer-integrated spin-valley microcavities, ±K' valley excitons couple to ±K spin-valley states owing to polarization matching, and spin-optical excitonic lasing is achieved at room tempera­tures through strong optical feedback. Meanwhile, ±K' valley excitons are driven by the lasing mechanism to find the minimum-loss state of the system, which leads them to re-establish a phase-locked correlation according to the opposite geometric phases of ±K spin-valley states. This lasing-mechanism-driven valley coherence removes the need for cryogenic temperatures to suppress the intervalley scattering. Moreover, the minimum-loss state of the Rashba monolayer laser can be regulated to be satisfied (broken) via a linear (circular) pump polari­zation, which provides a way to control the lasing intensity and spatial coherence.

“The unveiled photonic spin valley Rashba effect provides a general mechanism to construct surface-emitting spin-optical light sources. The demonstrated valley coherence in the monolayer-integrated spin–valley micro­cavity makes a step towards achieving entangle­ment between ±K' valley excitons for quantum information by means of qubits,” explains Hasman. “For a long time, our group has been working on deve­loping spin optics to harness photonic spin as an effective tool to control the behavior of electromagnetic waves. In 2018, we were attracted by valley pseudospins in two-dimensional materials, and therefore began a long-term project to study the active control of atomic-scale spin-optical light sources in the absence of magnetic fields. We initially tackled the challenge of coherent geometric phase pickup from individual valley excitons by using a non-local Berry-phase defect mode. However, the underlying coherent addition of multiple valley excitons of the realized Rashba monolayer light sources remained unsolved, owing to the lack of a strong synchroni­zing mechanism between the excitons. This issue inspired us to think about high-Q photonic Rashba modes. Following inno­vations in new physical approaches, we achieved the Rashba monolayer laser described here.” (Source: Technion)

Reference: K. Rong et al.: Spin-valley Rashba monolayer laser, Nat. Mat. 22, 1085 (2023); DOI: 10.1038/s41563-023-01603-3

Link: Atomic-Scale Photonics Laboratory, Technion – Israel Institute of Technology, Haifa, Israel